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Polarization-tuneable excitonic spectral features in the optoelectronic response of atomically thin ReS2

dc.contributor.authorVaquero D
dc.contributor.authorArroyo-Gascón O
dc.contributor.authorSalvador-Sánchez J
dc.contributor.authorAlcázar-Ruano P.L
dc.contributor.authorDiez E
dc.contributor.authorPerez-Rodríguez A
dc.contributor.authorCorrea J.D
dc.contributor.authorDominguez-Adame F
dc.contributor.authorChico L
dc.contributor.authorQuereda J.
dc.date.accessioned2024-07-31T21:07:03Z
dc.date.available2024-07-31T21:07:03Z
dc.date.created2024
dc.identifier.issn20531583
dc.identifier.urihttp://hdl.handle.net/11407/8460
dc.descriptionThe low crystal symmetry of rhenium disulphide (ReS2) leads to the emergence of dichroic optical and optoelectronic response, absent in other layered transition metal dichalcogenides, which could be exploited for device applications requiring polarization resolution. To date, spectroscopy studies on the optical response of ReS2 have relied almost exclusively in characterization techniques involving optical detection, such as photoluminescence, absorbance, or reflectance spectroscopy. However, to realize the full potential of this material, it is necessary to develop knowledge on its optoelectronic response with spectral resolution. In this work, we study the polarization-dependent photocurrent spectra of few-layer ReS2 photodetectors, both in room conditions and at cryogenic temperature. Our spectral measurements reveal two main exciton lines at energies matching those reported for optical spectroscopy measurements, as well as their excited states. Moreover, we also observe an additional exciton-like spectral feature with a photoresponse intensity comparable to the two main exciton lines. We attribute this feature, not observed in earlier photoluminescence measurements, to a non-radiative exciton transition. The intensities of the three main exciton features, as well as their excited states, modulate with linear polarization of light, each one acquiring maximal strength at a different polarization angle. We have performed first-principles exciton calculations employing the Bethe-Salpeter formalism, which corroborate our experimental findings. Our results bring new perspectives for the development of ReS2-based nanodevices. © 2023 The Author(s). Published by IOP Publishing Ltd.
dc.language.isoeng
dc.publisherInstitute of Physics
dc.relation.isversionofhttps://www.scopus.com/inward/record.uri?eid=2-s2.0-85177555049&doi=10.1088%2f2053-1583%2fad0402&partnerID=40&md5=7d49c2cfdef6421e76c11b64456ebb19
dc.source2D Materials
dc.source2D Materials
dc.sourceScopus
dc.subjectExcitoneng
dc.subjectOptoelectronicseng
dc.subjectPhotocurrent spectroscopyeng
dc.subjectPolarization-dependenteng
dc.subjectReS2eng
dc.subjectCrystal symmetryeng
dc.subjectExcited stateseng
dc.subjectExcitonseng
dc.subjectPhotoluminescenceeng
dc.subjectPolarizationeng
dc.subjectRhenium compoundseng
dc.subjectTransition metalseng
dc.subjectDevice applicationeng
dc.subjectExcited-stateseng
dc.subjectExciton lineseng
dc.subjectExcitonicseng
dc.subjectLayered transition metal dichalcogenideseng
dc.subjectOptical responseeng
dc.subjectOptical-eng
dc.subjectPhotocurrent spectroscopyeng
dc.subjectPolarization-dependenteng
dc.subjectSpectral featureeng
dc.subjectSulfur compoundseng
dc.titlePolarization-tuneable excitonic spectral features in the optoelectronic response of atomically thin ReS2eng
dc.typearticle
dc.rights.accessrightsinfo:eu-repo/semantics/restrictedAccess
dc.type.spaArtículo
dc.identifier.doi10.1088/2053-1583/ad0402
dc.relation.citationvolume11
dc.relation.citationissue1
dc.publisher.facultyFacultad de Ciencias Básicasspa
dc.affiliationVaquero, D., Nanotechnology Group, USAL-Nanolab, Universidad de Salamanca, Salamanca, E-37008, Spain
dc.affiliationArroyo-Gascón, O., Instituto de Ciencia de Materiales de Madrid, CSIC, Madrid, E-28049, Spain, Departamento de Física de Materiales, GISC, Universidad Complutense de Madrid, Madrid, E-28040, Spain
dc.affiliationSalvador-Sánchez, J., Nanotechnology Group, USAL-Nanolab, Universidad de Salamanca, Salamanca, E-37008, Spain
dc.affiliationAlcázar-Ruano, P.L., Departamento de Física de Materiales, GISC, Universidad Complutense de Madrid, Madrid, E-28040, Spain
dc.affiliationDiez, E., Nanotechnology Group, USAL-Nanolab, Universidad de Salamanca, Salamanca, E-37008, Spain
dc.affiliationPerez-Rodríguez, A., Nanotechnology Group, USAL-Nanolab, Universidad de Salamanca, Salamanca, E-37008, Spain
dc.affiliationCorrea, J.D., Facultad de Ciencias Básicas, Universidad de Medellín, Medellín, Colombia
dc.affiliationDominguez-Adame, F., Departamento de Física de Materiales, GISC, Universidad Complutense de Madrid, Madrid, E-28040, Spain
dc.affiliationChico, L., Departamento de Física de Materiales, GISC, Universidad Complutense de Madrid, Madrid, E-28040, Spain
dc.affiliationQuereda, J., Departamento de Física de Materiales, GISC, Universidad Complutense de Madrid, Madrid, E-28040, Spain
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dc.type.versioninfo:eu-repo/semantics/publishedVersion
dc.identifier.reponamereponame:Repositorio Institucional Universidad de Medellín
dc.identifier.repourlrepourl:https://repository.udem.edu.co/
dc.identifier.instnameinstname:Universidad de Medellín


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