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Dry-co-grinding of doped TiO2 with nitrogen, silicon or selenium for enhanced photocatalytic activity under UV/visible and visible light irradiation for environmental applications
dc.creator | Galeano L. | |
dc.creator | Valencia S. | |
dc.creator | Restrepo G. | |
dc.creator | Marín J.M. | |
dc.date | 2019 | |
dc.date.accessioned | 2021-02-05T14:59:04Z | |
dc.date.available | 2021-02-05T14:59:04Z | |
dc.identifier.issn | 13698001 | |
dc.identifier.uri | http://hdl.handle.net/11407/6067 | |
dc.description | TiO2 doped with nitrogen (N), silicon (Si), or selenium (Se) (N-TiO2, Si-TiO2, and Se-TiO2) were obtained by the integrated sol-gel and solvothermal method with short time of crystallization and low temperature. The UV/visible and visible light absorption and photocatalytic activity of these doped TiO2 materials were improved by a dry-co-grinding process with a short grinding time and low rotational speed (30 min at 200 rpm) to obtain N-TiO2/Si-TiO2 and N-TiO2/Se-TiO2 catalysts. The materials were characterized by XRD, Raman, BET surface area and porosity, XRF, SEM, TEM, FTIR-ATR, and UV/vis-DRS analyses. The photocatalytic activity of these materials was evaluated by the degradation of phenol under UV/visible and visible light irradiation. The integrated sol-gel and solvothermal methods with short time of crystallization (2 h) and low temperature (225 °C), and the dry-co-grinding process during 30 min at 200 rpm led to materials (N-TiO2/Si-TiO2 and N-TiO2/Se-TiO2) with higher specific surface area, a reduction in the band gap value, and an enhancement of the absorption in the visible light spectrum. Moreover, N-TiO2/Si-TiO2 and N-TiO2/Se-TiO2 exhibited higher photocatalytic activities for degradation of phenol under UV/visible and visible light irradiation than those obtained with the doped TiO2, synthesized TiO2 or TiO2 P25. © 2018 Elsevier Ltd | |
dc.language.iso | eng | |
dc.publisher | Elsevier Ltd | |
dc.relation.isversionof | https://www.scopus.com/inward/record.uri?eid=2-s2.0-85056447917&doi=10.1016%2fj.mssp.2018.10.032&partnerID=40&md5=6f1257beec245a025044bbf8ddc0b7c3 | |
dc.source | Materials Science in Semiconductor Processing | |
dc.title | Dry-co-grinding of doped TiO2 with nitrogen, silicon or selenium for enhanced photocatalytic activity under UV/visible and visible light irradiation for environmental applications | |
dc.type | Article | eng |
dc.rights.accessrights | info:eu-repo/semantics/restrictedAccess | |
dc.publisher.program | Ingeniería Ambiental | spa |
dc.identifier.doi | 10.1016/j.mssp.2018.10.032 | |
dc.relation.citationvolume | 91 | |
dc.relation.citationstartpage | 47 | |
dc.relation.citationendpage | 57 | |
dc.publisher.faculty | Facultad de Ingenierías | spa |
dc.affiliation | Galeano, L., Grupo de Investigaciones y Mediciones Ambientales (GEMA), Universidad de Medellín, Carrera 87 No 30-65, Medellín, Colombia, Grupo Procesos Fisicoquímicos Aplicados, Departamento de Ingeniería Química, Facultad de Ingeniería, Sede de Investigación Universit:aria, Universidad de Antioquia UdeA, Calle 70 No. 52-21, Medellín, Colombia | |
dc.affiliation | Valencia, S., Grupo de investigación Integra, Tecnológico de Antioquia, Calle 78B No 72A-220, Medellín, Colombia, Grupo Procesos Fisicoquímicos Aplicados, Departamento de Ingeniería Química, Facultad de Ingeniería, Sede de Investigación Universit:aria, Universidad de Antioquia UdeA, Calle 70 No. 52-21, Medellín, Colombia | |
dc.affiliation | Restrepo, G., Grupo Procesos Fisicoquímicos Aplicados, Departamento de Ingeniería Química, Facultad de Ingeniería, Sede de Investigación Universit:aria, Universidad de Antioquia UdeA, Calle 70 No. 52-21, Medellín, Colombia | |
dc.affiliation | Marín, J.M., Grupo Procesos Fisicoquímicos Aplicados, Departamento de Ingeniería Química, Facultad de Ingeniería, Sede de Investigación Universit:aria, Universidad de Antioquia UdeA, Calle 70 No. 52-21, Medellín, Colombia | |
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dc.type.version | info:eu-repo/semantics/publishedVersion | |
dc.type.driver | info:eu-repo/semantics/article |
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