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Production of activated carbon from agave residues and its synergistic application in a hybrid adsorption-AOPs system for effective removal of sulfamethazine from aqueous solutions

dc.contributor.authorSerna-Carrizales J.C
dc.contributor.authorZárate Guzmán A.I
dc.contributor.authorForgionny A
dc.contributor.authorAcelas N
dc.contributor.authorPérez S
dc.contributor.authorMuñoz-Saldaña J
dc.contributor.authorOcampo-Perez R.
dc.date.accessioned2024-07-31T21:07:03Z
dc.date.available2024-07-31T21:07:03Z
dc.date.created2024
dc.identifier.issn139351
dc.identifier.urihttp://hdl.handle.net/11407/8461
dc.descriptionTequila production in Mexico generates large quantities of agave bagasse (AB), a waste that could be used more efficiently. AB has a high cellulose, hemicellulose, and lignin content, which allows its use as a precursor for synthesizing carbonaceous materials. In the present work, the synthesis of activated carbon impregnated with Fe2+ (AG-Fe-II) and Fe3+ (AG-Fe-III) was carried out and evaluated in a hybrid adsorption-AOP (advanced oxidation process) methodology for sulfamethazine removal (SMT). The materials were characterized before and after the process to determine their morphological, textural, and physicochemical properties. Subsequently, the effect of the main operational variables (pH, initial SMT concentration, mass, and activator dosage) on the hybrid adsorption-degradation process was studied. The Fenton-like reaction was selected as the AOP for the degradation step, and potassium persulfate (K2S2O8) was used as an activating agent. The main iron crystallographic phases in AG-Fe-II were FeS, with a uniform distribution of iron particles over the material's surface. The main crystallographic phase for AG-Fe-III was Fe3O4. The hybrid process achieved 61% and 78% removal efficiency using AG-Fe-II and AG-Fe-III samples, respectively. The pH and initial SMT concentration were the most critical factors for removing SMT from an aqueous phase. Finally, the material was successfully tested in repeated adsorption-degradation cycles. © 2024 Elsevier Inc.
dc.language.isoeng
dc.publisherAcademic Press Inc.
dc.relation.isversionofhttps://www.scopus.com/inward/record.uri?eid=2-s2.0-85186271268&doi=10.1016%2fj.envres.2024.118559&partnerID=40&md5=fc8294f6cf1ae99d81960b83203c9f4b
dc.sourceEnvironmental Research
dc.sourceEnviron. Res.
dc.sourceScopus
dc.subjectAdsorptioneng
dc.subjectAdvanced oxidation processeng
dc.subjectAgave residueseng
dc.subjectFenton processeng
dc.subjectSulfamethazineeng
dc.subjectActivated carboneng
dc.subjectCelluloseeng
dc.subjectMagnetiteeng
dc.subjectOxidationeng
dc.subjectPhysicochemical propertieseng
dc.subjectPotassium compoundseng
dc.subjectSilver compoundseng
dc.subjectAdvanced Oxidation Processeseng
dc.subjectAgave bagasseeng
dc.subjectAgave residueeng
dc.subjectCellulose contenteng
dc.subjectCrystallographic phaseeng
dc.subjectEffective removalseng
dc.subjectFenton's processeng
dc.subjectLignin contentseng
dc.subjectMe-xicoeng
dc.subjectSulfamethazineeng
dc.subjectAdsorptioneng
dc.titleProduction of activated carbon from agave residues and its synergistic application in a hybrid adsorption-AOPs system for effective removal of sulfamethazine from aqueous solutionseng
dc.typearticle
dc.rights.accessrightsinfo:eu-repo/semantics/restrictedAccess
dc.type.spaArtículo
dc.identifier.doi10.1016/j.envres.2024.118559
dc.relation.citationvolume250
dc.publisher.facultyFacultad de Ciencias Básicasspa
dc.affiliationSerna-Carrizales, J.C., Centro de Investigación y Estudios de Posgrado, Facultad de Ciencias Químicas, Universidad Autónoma de San Luis Potosí, San Luis Potosí, 78260, Mexico
dc.affiliationZárate Guzmán, A.I., Centro de Investigación y Estudios de Posgrado, Facultad de Ciencias Químicas, Universidad Autónoma de San Luis Potosí, San Luis Potosí, 78260, Mexico, Grupo de Investigación en Materiales y Fenómenos de Superficie, Departamento de Biotecnológicas y Ambientales, Universidad Autónoma de Guadalajara, Av. Patria 1201, Zapopan, 45129, Mexico
dc.affiliationForgionny, A., Grupo de Investigación Materiales con Impacto (Mat&mpac), Facultad de Ciencias Básicas, Universidad de Medellín, Carrera 87 No. 30-65, Medellín, 050026, Colombia
dc.affiliationAcelas, N., Grupo de Investigación Materiales con Impacto (Mat&mpac), Facultad de Ciencias Básicas, Universidad de Medellín, Carrera 87 No. 30-65, Medellín, 050026, Colombia
dc.affiliationPérez, S., Laboratorio Nacional de Proyección Térmica (CENAPROT), Centro de Investigación y de Estudios Avanzados del IPN, Libramiento Norponiente 2000 Fracc, Real de Juriquilla, Querétaro, 76230, Mexico
dc.affiliationMuñoz-Saldaña, J., Laboratorio Nacional de Proyección Térmica (CENAPROT), Centro de Investigación y de Estudios Avanzados del IPN, Libramiento Norponiente 2000 Fracc, Real de Juriquilla, Querétaro, 76230, Mexico
dc.affiliationOcampo-Perez, R., Centro de Investigación y Estudios de Posgrado, Facultad de Ciencias Químicas, Universidad Autónoma de San Luis Potosí, San Luis Potosí, 78260, Mexico
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dc.type.versioninfo:eu-repo/semantics/publishedVersion
dc.identifier.reponamereponame:Repositorio Institucional Universidad de Medellín
dc.identifier.repourlrepourl:https://repository.udem.edu.co/
dc.identifier.instnameinstname:Universidad de Medellín


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