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Understanding mechanisms in the adsorption of lead and copper ions on chili seed waste in single and multicomponent systems: a combined experimental and computational study

dc.creatorForgionny A.
dc.creatorAcelas N.Y.
dc.creatorOcampo-Pérez R.
dc.creatorPadilla-Ortega E.
dc.creatorLeyva-Ramos R.
dc.creatorFlórez E.
dc.date2021
dc.date.accessioned2021-02-05T14:57:40Z
dc.date.available2021-02-05T14:57:40Z
dc.identifier.issn9441344
dc.identifier.urihttp://hdl.handle.net/11407/5901
dc.descriptionIn the current work, a deep study to understand the adsorption phenomena occurring in single and multicomponent systems was conducted by using spectroscopic characterization, and computational tools. The experimental results showed that the adsorption capacity of chili seed is higher for Pb2+ (48 mg/g) than Cu2+ (4.1 mg/g) ions in single systems. However, the adsorption study in multicomponent systems provides important conclusions of the concentration effect of the metal ions, showing a significant antagonistic and competitive effect of both ions under equivalent concentrations of them (qPb2+ is 56% reduced) or high concentration of Pb2+ (qCu2+ is 50% reduced). Computational results correlated well with the experimental ones and evidenced all interactions proposed from spectroscopy results, accounting for the occurrence of complexation and electrostatic mechanisms between metal ions and the surface oxygenated functional groups (hydroxyl, carboxyl, and carboxylate) onto chili seed. Chemistry quantum descriptors supported the reactivity behavior of the chemical species implicated. All results evidenced that Pb2+ and Cu2+ adsorption on chili seed surface is governed by the occurrence of combined ionic exchange, π-interaction, complexation, and electrostatic attraction. © 2021, Springer-Verlag GmbH Germany, part of Springer Nature.
dc.language.isoeng
dc.publisherSpringer Science and Business Media Deutschland GmbH
dc.relation.isversionofhttps://www.scopus.com/inward/record.uri?eid=2-s2.0-85099459696&doi=10.1007%2fs11356-020-11721-z&partnerID=40&md5=9140850629dba41dd6ec7896a3db59b2
dc.sourceEnvironmental Science and Pollution Research
dc.subjectAdsorptionspa
dc.subjectCopperspa
dc.subjectLeadspa
dc.subjectMechanismspa
dc.subjectMulticomponentspa
dc.subjectSinglespa
dc.titleUnderstanding mechanisms in the adsorption of lead and copper ions on chili seed waste in single and multicomponent systems: a combined experimental and computational study
dc.typeArticleeng
dc.rights.accessrightsinfo:eu-repo/semantics/restrictedAccess
dc.identifier.doi10.1007/s11356-020-11721-z
dc.publisher.facultyFacultad de Ciencias Básicasspa
dc.affiliationForgionny, A., Grupo de Materiales con Impacto, Mat&mpac. Facultad de Ciencias Básicas, Universidad de Medellín, Medellín, Colombia
dc.affiliationAcelas, N.Y., Grupo de Materiales con Impacto, Mat&mpac. Facultad de Ciencias Básicas, Universidad de Medellín, Medellín, Colombia
dc.affiliationOcampo-Pérez, R., Centro de Investigación y Estudios de Posgrado, Facultad de Ciencias Químicas, Universidad Autónoma de San Luis Potosi, San Luis Potosi, 78260, Mexico
dc.affiliationPadilla-Ortega, E., Centro de Investigación y Estudios de Posgrado, Facultad de Ciencias Químicas, Universidad Autónoma de San Luis Potosi, San Luis Potosi, 78260, Mexico
dc.affiliationLeyva-Ramos, R., Centro de Investigación y Estudios de Posgrado, Facultad de Ciencias Químicas, Universidad Autónoma de San Luis Potosi, San Luis Potosi, 78260, Mexico
dc.affiliationFlórez, E., Grupo de Materiales con Impacto, Mat&mpac. Facultad de Ciencias Básicas, Universidad de Medellín, Medellín, Colombia
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